Journal
PHYSICAL REVIEW LETTERS
Volume 98, Issue 23, Pages -Publisher
AMER PHYSICAL SOC
DOI: 10.1103/PhysRevLett.98.235503
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Coherent anti-Stokes Raman spectroscopy has been used to study deuterium at ambient temperature to 187 GPa, the highest pressure this technique has ever been applied. The pressure dependence of the nu(1) vibron line shape indicates that deuterium has a rho(direct)=0.501 and rho(exciton)=0.434 mol/cm(3) for a band gap of 2 omega(P)=4.66 eV. The extrapolation from the ambient pressure band gap yields a metallization pressure of 460 GPa, confirming earlier measurements. Above 143 GPa, the Raman shift data provide clear evidence for the presence of the ab initio predicted I-' phase of deuterium.
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