Journal
TETRAHEDRON
Volume 63, Issue 26, Pages 6035-6041Publisher
PERGAMON-ELSEVIER SCIENCE LTD
DOI: 10.1016/j.tet.2007.02.115
Keywords
carbon-phosphorus ylide; phosphine; allylic compounds; 2-substituted 1,1-dicyanoalkenes
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A highly regio-and stereo-selective phosphine-catalyzed [3+ 2] annulation reaction between allylic compounds and 2-substituted 1,1-dicyanoalkenes through a catalytic phosphorus ylide reaction was developed. This reaction has the total reversed regioselectivity compared to that of the reactions of activated alkenes without the 2-substituents or reactions using the allenoates as the C3 component. (c) 2007 Elsevier Ltd. All rights reserved.
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