Journal
ANALYTICAL AND BIOANALYTICAL CHEMISTRY
Volume 400, Issue 9, Pages 3125-3132Publisher
SPRINGER HEIDELBERG
DOI: 10.1007/s00216-011-4979-2
Keywords
Accelerator mass spectrometry; Long-lived radionuclides; Cosmogenic nuclides; Exposure dating
Funding
- INSU/CNRS
- French Ministry of Research and Higher Education
- IRD
- CEA
- CRONUS-EU [511927]
- Grants-in-Aid for Scientific Research [21310004] Funding Source: KAKEN
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A first international Cl-36 interlaboratory comparison has been initiated. Evaluation of the final results of the eight participating accelerator mass spectrometry (AMS) laboratories on three synthetic AgCl samples with Cl-36/Cl ratios at the 10(-11), 10(-12), and 10(-13) level shows no difference in the sense of simple statistical significance. However, more detailed statistical analyses demonstrate certain interlaboratory bias and underestimation of uncertainties by some laboratories. Following subsequent remeasurement and reanalysis of the data from some AMS facilities, the round-robin data indicate that Cl-36/Cl data from two individual AMS laboratories can differ by up to 17%. Thus, the demand for further work on harmonising the Cl-36-system on a worldwide scale and enlarging the improvement of measurements is obvious.
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