Journal
ORGANIC LETTERS
Volume 9, Issue 18, Pages 3647-3650Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ol7015274
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alpha,beta-Unsaturated 2-acyl imidazoles are a novel and practical class of dienophiles for the DNA-based catalytic asymmetric Diels-Alder reaction in water. The Diels-Alder products are obtained with very high diastereoselectivities and enantioselectivities in the range of 83-98%. The catalytic reaction was performed on a 1.0 mmol scale, and the imidazole auxiliary was removed readily.
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