Journal
ADVANCED SYNTHESIS & CATALYSIS
Volume 349, Issue 14-15, Pages 2241-2246Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/adsc.200700223
Keywords
arenes; carboxylic acids; catalysis; copper; decarboxylation
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A catalyst generated from copper(I) oxide and 4,7-diphenyl-1,10-phenanthroline for the first time allows the catalytic protodecarboxylation even of deactivated aromatic carboxylic acids, giving rise to the corresponding arenes. Based on DFT calculations, a reaction pathway is proposed that accurately reflects the experimental results, such as the observed reactivity order of the substrates.
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