Journal
JOURNAL OF ORGANIC CHEMISTRY
Volume 72, Issue 21, Pages 8135-8138Publisher
AMER CHEMICAL SOC
DOI: 10.1021/jo701431j
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[GRAPHICS] An efficient two-step strategy has been developed to access diversely functionalized benzylic sulfonamides. Execution of this strategy required the development of two reaction methods: the palladium-catalyzed cross-coupling of aryl halides with CH-acidic methanesulfonamides and a metathesis reaction between the resulting alpha-arylated sulfonamides and diverse amines. The broad scope of the cross-coupling process combined with a versatile sulfonamide metathesis constitutes an efficient strategy for the synthesis of various benzylic sulfonamides.
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