Journal
OPTICS LETTERS
Volume 32, Issue 20, Pages 2966-2968Publisher
OPTICAL SOC AMER
DOI: 10.1364/OL.32.002966
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Two-dimensional (2D) Fourier transform (FT) infrared spectroscopy is performed by using a collinear pulse-pair pump and probe geometry with conventional optics. Simultaneous collection of the third-order response and pulse-pair timing permit automated phasing and rapid acquisition of 2D absorptive spectra. To demonstrate the ability of this method to capture molecular dynamics, couplings and structure found in the conventional boxcar 2D) FT spectroscopy, a series of 2D) spectra of a metal carbonyl, and a beta-sheet protein are acquired. (C) 2007 Optical Society of America
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