Journal
CHEMICAL PHYSICS
Volume 341, Issue 1-3, Pages 89-94Publisher
ELSEVIER SCIENCE BV
DOI: 10.1016/j.chemphys.2007.06.027
Keywords
multidimensional spectroscopy; four-wave mixing; coherent; ultrafast spectroscopy; pulse shaping
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We have demonstrated a highly efficient fully coherent 2D spectrometer based on 2D pulse shaping and Fourier beam shaping. The versatility of the design allows one to measure different 2D spectral surfaces consecutively. Easy alignment, inherent phase stability, rotating wave frame detection, and arbitrary waveform generation in all of the beams are important features of this design. We have demonstrated the functionality of the 2D spectrometer by measuring a 2D spectral surface of a GaAs quantum well. (C) 2007 Elsevier B.V. All rights reserved.
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