Journal
ORGANIC LETTERS
Volume 9, Issue 24, Pages 4939-4942Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ol701962w
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The heterogeneous catalytic hydrogenation of highly substituted pyrrole systems was studied. These aromatic systems could be fully reduced with excellent diastereoselectivity to afford functionalized pyrrolidines with up to four new stereocenters. It is likely that the reaction is a two-step hydrogenation sequence, and that initial reduction of the C=X bond provides a stereocenter that directs the subsequent reduction of the pyrrole.
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