Journal
ORGANIC LETTERS
Volume 9, Issue 25, Pages 5283-5286Publisher
AMER CHEMICAL SOC
DOI: 10.1021/ol702447y
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The intramolecular aza-Michael reaction of carbamates bearing remote alpha,beta-unsaturated aldehydes under organocatalytic conditions took place with good yields and excellent ee's when Jorgensen catalyst IV was used in the process, giving rise to the enantioselective formation of several five- and six-membered heterocycles. The developed methodology was applied to the synthesis of three piperidine alkaloids.
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