Journal
ADVANCES IN WATER RESOURCES
Volume 33, Issue 4, Pages 361-371Publisher
ELSEVIER SCI LTD
DOI: 10.1016/j.advwatres.2009.12.001
Keywords
Nanoparticles; Mobility; Subsurface; Carbon nanotubes; nC(60)
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Funding
- Ontario Ministry of the Environment
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The production and use of nanomaterials will inevitably lead to their disposal in the natural environment. To assess the risk that these materials pose to human and ecosystem health an understanding of their mobility and ultimate fate is essential. To date, however, relatively little research has been conducted on the fate of nanoparticles in subsurface systems. In this study the subsurface mobility of two carbon nanoparticles: nano-fullerenes (nC(60)) and multi-walled carbon nanotubes (MWCNTs) is assessed. A two-dimensional finite element model was used to simulate the movement of these nanoparticles under a range of hydrologic and geological conditions, including a heterogeneous permeability field. The numerical model is based on colloid filtration theory (CFT) with a maximum retention capacity term. For the conditions evaluated the carbon nanotubes are much more mobile than nC(60) due to the smaller collector efficiency associated with carbon nanotubes. However, the mobility of nC(60) increased significantly when a maximum retention capacity term was included in the model. Model results also demonstrate that, for the systems examined, nanoparticles were predicted to be less mobile in heterogeneous systems compared to the homogeneous systems with the same average hydraulic properties. (C) 2010 Elsevier Ltd. All rights reserved.
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