Journal
ADVANCED SYNTHESIS & CATALYSIS
Volume 360, Issue 13, Pages 2470-2475Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/adsc.201800322
Keywords
Iridium(III) catalysts; C-H annulation; N-phenoxyacetamides; tertiary propargyl alcohols; benzofurans
Categories
Funding
- NSFC [81502909]
- Guangdong Natural Science Funds for Distinguished Young Scholar [2017A030306031]
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An efficient, mild and redox-neutral iridium(III)-catalyzed C-H annulation of N-phenoxyacetamides for the regioselective synthesis of benzofurans has been developed by employing tertiary propargyl alcohols as the versatile coupling partners. The computed results together with the experimental data revealed that the hydroxyl group of tertiary propargyl alcohols acts as the key factor in controlling the regioselectivity and tuning the reactivity.
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