Journal
ADVANCED SYNTHESIS & CATALYSIS
Volume 356, Issue 13, Pages 2749-2755Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/adsc.201400556
Keywords
amino acids; aminomethylation; electron transfer; photocatalysis; photochemistry
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Funding
- Ministry of Education, Culture, Sports, Science of the Japanese Government [26288045]
- Grants-in-Aid for Scientific Research [26288045] Funding Source: KAKEN
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A photocatalytic hydroaminomethylation of olefins with N-protected aminomethyltrifluoroborates has been developed. This methodology provides a new strategy for the introduction of a primary aminomethyl group onto electron-deficient C=C bonds. This reaction constitutes a facile entry into synthetically useful gamma-aminobutyric acid (GABA) derivatives such as baclofen.
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