Journal
ADVANCED SYNTHESIS & CATALYSIS
Volume 355, Issue 9, Pages 1748-1754Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/adsc.201300120
Keywords
dendrimers; magnetic nanoparticles; Michael addition; organocatalysis; recycling
Categories
Funding
- CNRS
- ANR
- Deutsche Forschungsgemeinschaft [Re 948/8-1]
- IDK NANO-CAT (Elitenetzwerk Bayern)
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The JOrgensen-Hayashi catalyst [(S)-,-diphenylprolinol trimethylsilyl ether] was grafted onto the surface of two different supports: phosphorus dendrimers (generations 1 to 3) and magnetic, polymer-coated cobalt/carbon (Co/C) nanobeads. These new supported catalysts displayed high activities and selectivities in the Michael additions of a wide range of aldehydes to different nitroolefins. Moreover, the dendrimer of the third generation displayed excellent recycling abilities since it could be recovered and reused in 7 consecutive runs without loss of activity.
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