Journal
ADVANCED SYNTHESIS & CATALYSIS
Volume 354, Issue 7, Pages 1293-1300Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/adsc.201100892
Keywords
copper; cross-coupling; dehydrogenation; oxidation; oxygen
Categories
Funding
- Peking University
- National Science Foundation of China [20872003]
- National Basic Research Program of China (973 Program) [2009CB825300]
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A novel copper-catalyzed, multiple oxidative dehydrogenative functionalization of arylacetaldehydes leading to 2-oxo-acetamidine compounds has been developed. This transformation is highly efficient with dissociation of six hydrogens including two sp3 C?H and one sp2 C?H bond activations. This method not only provides an efficient approach to 2-oxo-acetamidine compounds, but also offers a valuable mechanistic insight into this novel copper catalysis.
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