Journal
ADVANCED SYNTHESIS & CATALYSIS
Volume 354, Issue 8, Pages 1422-1428Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/adsc.201100926
Keywords
addition reaction; asymmetric synthesis; chiral additives; enantioselectivity; ketimines
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Funding
- National Natural Science Foundation of China (NSFC) [20972110, 21002068]
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A novel enantioselective diynylation of cyclic N-acyl trifluoromethylketimines with chloramphenicol-amine derivatives as chiral additives has been successfully developed. A series of diynylated tertiary trifluoromethylcarbinamines were obtained in high yields with good to excellent enantioselectivities (with up to 99% ee).
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