Journal
ADVANCED SYNTHESIS & CATALYSIS
Volume 352, Issue 1, Pages 97-102Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/adsc.200900657
Keywords
activated alkenes; cascade reactions; multicomponent reactions; nitromethane; organocatalysis
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Funding
- National Natural Science Foundation of China [20672057, 20872063]
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A new tertiary amine-catalyzed cascade Michael-Michael-Henry reaction between nitromethane, a doubly activated alkene and an alpha,beta-unsaturated carbonyl compound is described, which provides a convenient and efficient synthesis for densely functionalized cyclohexanes and some bicyclic compounds in moderate to excellent yields with high diastereoselectivity.
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