Journal
ADVANCED SYNTHESIS & CATALYSIS
Volume 352, Issue 7, Pages 1145-1149Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/adsc.200900874
Keywords
acylation; aliphatic aldehydes; C-H functionalization; oxidative cross-coupling; palladium catalysis
Categories
Funding
- Canada Research Chair (Tier 1) Foundation
- NSERC
- Canada Foundation for Innovation (CFI)
- FQRNT
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An efficient method was developed for the direct acylation of arene sp(2) C-H bonds with aldehydes using palladium acetate as catalyst and peroxide as oxidant. The solvent-free oxidative acylation reaction assisted by a pyridine directing group provides an easy access to aromatic, aliphatic, and optical active ketones.
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