Journal
ADVANCED MATERIALS
Volume 26, Issue 32, Pages 5613-+Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/adma.201401182
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Funding
- Ministry of Science and Technology of China [2013CB834505, 2014CB239402]
- National Natural Science Foundation of China [91127005, 51322213, 51172245, 20901081]
- Chinese Academy of Sciences [KGCX2-EW-311-3]
- Ten Thousand Talents Plan
- 100 Talents Program of the Chinese Academy of Sciences
- University of Maryland
- National Science Foundation [2012143497]
- National Natural Science Foundation for Distinguished Youth Scholars of China [21025310]
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A novel versatile light-triggered strategy is developed to organize inorganic nanoparticles (NPs) into nanovesicles with single or multiple layers in mixed solvents. This strategy constitutes a new assembly mechanism based on the photo-oxidation of thiol ligands. Compared with currently-used individual semiconductor NPs, the prepared CdSe QD vesicles exhibit an improved catalytic activity and unprecedented catalytic stability towards solar-driven hydrogen production. This light-triggered approach to functional nanoarchitectures would lead to new opportunities in various applications.
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