Journal
ADVANCED MATERIALS
Volume 26, Issue 40, Pages 6912-6920Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/adma.201305317
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Funding
- National Key Project on Basic Research [2011CB808700, 2011CB932300]
- National Natural Science Foundation of China [91023013, 21121063, 21127901]
- Chinese Academy of Sciences
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Two-dimensional (2D) nanomaterials, such as graphene and transition metal chalcogenides, show many interesting dimension-related materials properties. Inspired by the development of 2D inorganic nanomaterials, single-layered covalent organic frameworks (sCOFs), featuring atom-thick sheets and crystalline extended organic structures with covalently bonded building blocks, have attracted great attention in recent years. With their unique graphene-like topological structure and the merit of structural diversity, sCOFs promise to possess novel and designable properties. However, the synthesis of sCOFs with well-defined structures remains a great challenge. Herein, the recent development of the bottom-up synthesis methods of 2D sCOFs, such as thermodynamic equilibrium control methods, growth-kinetics control methods, and surface-assisted covalent polymerization methods, are reviewed. Finally, some of the critical properties and application prospects of these materials are outlined.
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