Journal
ADVANCED MATERIALS
Volume 25, Issue 14, Pages 2084-2089Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/adma.201204237
Keywords
organic microfibers; nonlinear optics; second harmonic generation; two-photon excited fluorescence; self-assembly
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Funding
- National Basic Research 973 Program of China [2011CB932302]
- National Nature Science Foundation of China [21031006]
- Netherlands Organization for Scientific Research (NWO)
- EC Marie- Curie ITN-SUPERIOR
- EC Marie-Curie ITN-HIERACHY
- VICI
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While highly desired in integrated optical circuits, multiresponsive and tunable nonlinear optical (NLO) active 1D (sub) wavelength scale superstructures from organic materials are rarely reported due to the strong tendency of organic molecules to self-assembly in centrosymmetric modes. Here a solution-processed assembly approach is reported to generate non-centrosymmetric single-crystalline organic microfibers with a cumulative dipole moment for anisotropic combined second-and third-order NLO.
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