Journal
ADVANCED MATERIALS
Volume 25, Issue 12, Pages 1761-1767Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/adma.201204240
Keywords
bilayers; compositionally graded heterostructures; built-in potential; ferroelectric domain structures; dielectric and ferroelectric properties
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Funding
- Defense Advanced Research Projects Agency (DARPA) [N66001-11-1-4195]
- Office of Naval Research [N00014-10-10525]
- Army Research Office [W911NF-10-1-0482]
- Air Force Office of Scientific Research [AF FA 9550-11-1-0073]
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Synthesis of compositionally graded versions of PbZr1-xTixO3 thin films results in unprecedented strains ( as large as approximate to 4.5 x 10(5) m(-1)) and correspondingly unexpected crystal structures, ferroelectric domain structures, and properties. This includes the observation of built-in electric fields in films as large as 200 kV/cm. Compositional and strain gradients could represent a new direction of strain-control of materials.
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