Journal
ADVANCED MATERIALS
Volume 25, Issue 4, Pages 635-639Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/adma.201203383
Keywords
hydrogen isotopes; gas adsorption; quantum sieving; isotope separation; metal-organic frameworks
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Funding
- DFG [SPP 1362]
- European Commission through an ERC Starting Grant [GA 256962]
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The metal-organic framework, MFU-4, possessing small cavities and apertures, is exploited for quantum sieving of hydrogen isotopes. Quantum mechanically, a molecule confined in a small cavity shows an increase in effective size depending on the particle mass, which leads to a faster deuterium adsorption from a H-2/D-2 isotope mixture.
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