Journal
ADVANCED MATERIALS
Volume 24, Issue 48, Pages 6473-6478Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/adma.201202525
Keywords
stimulated resonance raman scattering; laser oscillations; amplified spontaneous emission; polarization; crystal structure; p-conjugated molecular crystals
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Funding
- Spanish Ministerio de Economia y Competitividad (MINECO) [CTQ2011-27317]
- Comunidad de Madrid [S2009/MAT-1726]
- EC [229599]
- MINECO [MAT2008-06648-C02, MAT2011-28167-C02]
- EC (FEDER)
- UA [GRE10-07]
- Basic Science Research Program (CRI) [RIAMI-AM0209(0417-20090011)]
- WCU (World Class University) project through National Research Foundation of Korea [R31-2008-000-10075-0]
- Ministry of Education, Science and Technology
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Three-in-one: A novel distyrylbenzene-based material forms J-type aggregates in single crystals with highly polarized and bright red emission, giving rise to optical gain narrowing, for which different mechanisms (amplified spontaneous emission, laser emission and stimulated resonance Raman scattering) are observed. These are correlated with the favorable intrinsic and macroscopic properties of the crystal, in particular to the orientation of the molecules to the crystal surface.
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