Journal
ADVANCED FUNCTIONAL MATERIALS
Volume 24, Issue 9, Pages 1228-1233Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/adfm.201302320
Keywords
electrochromic polymers; electrochromic devices; PEDOT:PSS; silver grid electrodes; ITO free
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Indium-doped tin oxide free electrochromic devices are prepared by coating electrochromic polymers onto polyethylene terephthalate substrates encompassing two different silver grids as electrodes. One design comprises a flexoprinted highly conductive silver grid electrode, yielding electrochromic devices with a response time of 2 s for an optical contrast of 27%. The other design utilizes an embedded silver grid electrode whereupon response times of 0.5 s for a 30% optical contrast are realized when oxidizing the device. A commercially available conductive poly(3,4-ethylenedioxythiophene):poly(4-styrenesulfonate acid) formulation (PEDOT:PSS) is coated onto the silver grids as a charge balancing polymer, and is in this setting found to be superior to a polypyrrole previously employed in electrochromic devices. In addition, the PEDOT:PSS layer increases the conductivity in the hexagonal grid structure.
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