Journal
ADVANCED FUNCTIONAL MATERIALS
Volume 23, Issue 43, Pages 5429-5435Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/adfm.201300495
Keywords
flexible electrode; Li4Ti5O12; lithium ion battery; nanosheets
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Funding
- Ministry of Science and Technology of China [2011CB932604]
- National Science Foundation of China [50921004, 51172239]
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Flexible energy-storage devices have attracted growing attention with the fast development of bendable electronic systems. Thus, the search for reliable electrodes with both high mechanical flexibility and excellent electron and lithium-ion conductivity has become an urgent task. Carbon-coated nanostructures of Li4Ti5O12 (LTO) have important applications in high-performance lithium ion batteries (LIBs). However, these materials still need to be mixed with a binder and carbon black and pressed onto metal substrates or, alternatively, by be deposited onto a conductive substrate before they are assembled into batteries, which makes the batteries less flexible and have a low energy density. Herein, a simple and scalable process to fabricate LTO nanosheets with a N-doped carbon coating is reported. This can be assembled into a film which can be used as a binder-free and flexible electrode for LIBs that does not require any current collectors. Such a flexible electrode has a long life. More significantly, it exhibits an excellent rate capability due to the thin carbon coating and porous nanosheet structures, which produces a highly conductive pathway for electrons and fast transport channels for lithium ions.
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