Journal
ADVANCED FUNCTIONAL MATERIALS
Volume 21, Issue 5, Pages 927-931Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/adfm.201002518
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Funding
- DHS [2009-DN-077-ARI028-03]
- NSF [DMR05-20415]
- Karlsruhe House of Young Scientists (KHYS)
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We demonstrate a novel approach for enhancing photoconductive responsivity (R) using a solution-based organic semiconductor composite that yields R approaching 25 AW(-1), which is two to three orders of magnitude higher than the R in films comprising a single molecular component. We present extensive studies of photoconductivity, photoluminescence, and crystalline structural order that elucidate the mechanisms underlying this high photoconductive responsivity. The high R is found to arise from high photoconductive gain (82) due to a long mobile hole lifetime stemming from a prolonged occupation of electrons in deep traps generated at interfacial regions between the molecular crystallites.
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