Journal
ADVANCED FUNCTIONAL MATERIALS
Volume 19, Issue 8, Pages 1207-1214Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/adfm.200801419
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Funding
- European Union through the Marie-Curie RTNs PRAIRIES [MRTN-CT-2006-035810]
- EST-SUPER [MEST-CT-2004-008128]
- MIUR [Firb RBIN04HC3S]
- Belgian National Research Foundation (FRS-FNRS) [2.4.625.08, 2.4.550.09]
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Here, the formation of discrete supramolecular mono- and bi-component architectures from novel and multivalent molecular modules bearing complementary recognition moieties that are prone to undergo multiple H-bonds, such as 2,6-di(acetylamino)pyridine and uracil residues, is described. These nanostructured H-bonded arrays, including dimeric and pentameric species, are thoroughly characterized in solution by NMR, in the solid state by FT-IR, and at the solid-liquid interface by means of scanning tunneling microscopy. The employed strategy is extremely versatile as it relies on the tuning of the valency, size, and geometry of the molecular modules; thus, it may be of interest for the bottom-up fabrication of nanostructured functional materials with sub-nanometer precision.
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