Journal
INORGANIC CHEMISTRY
Volume 54, Issue 23, Pages 11520-11525Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acs.inorgchem.5b02196
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Funding
- National Natural Science Foundation of China [21373162, 21203149, 21127004, 21173168, 21463020]
- Nature Science Foundation of Shaanxi Province [11JS110, FF10091, SJ08B09]
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A three-dimensional metal-organic framework based, high-energy-density compound, [Co-5(3-atrz)(7)(N-3)(3)] (3-atrz = 3-amine-1H-1,2,4-triazole), features superior detonation properties, insensitivity, and thermostability. Magnetic studies show that the compound characterizes the coexistence of remarkable coercivity, metamagnetism, long-range ordering, and relaxation dynamics. The heat-capacity measurement confirms the typical long-range antiferromagnetic ordering below 16 K. This difunctional system exemplifies an effective attempt at developing advanced magnetoenergetic materials.
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