Journal
INORGANIC CHEMISTRY
Volume 54, Issue 8, Pages 4138-4142Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acs.inorgchem.5b00401
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Funding
- NSFC [21371147, 21365021, 51172277, U1129301]
- XJSF [2013711009, 2013211A026]
- Xinjiang International Science & Technology Cooperation Program [20146001]
- Funds for Creative Cross & Cooperation Teams of CAS
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The first borate carbonate UV nonlinear optical material Pb7O(OH)(3)(CO3)(3)(BO3) was hydrothermally synthesized, which features a (3,9)-connected IrSi3-like structure constructed by Pb7O(OH)(3)(BO3) units and carbonates. This compound exhibits a large second-harmonic generation (SHG) response about 4.5 times that of KH2PO4 (KDP), attributed to synergistic interactions between the stereoeffect of the Pb(II) cations and coparallel BO3 and CO3 triangles groups.
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