Journal
ACS NANO
Volume 8, Issue 7, Pages 7147-7155Publisher
AMER CHEMICAL SOC
DOI: 10.1021/nn502115k
Keywords
perovskite; solar cells; mobility; traps; doping
Categories
Funding
- European Union [316494]
- Engineering and Physical Sciences Research Council [1511477, EP/G049653/1] Funding Source: researchfish
- EPSRC [EP/G049653/1] Funding Source: UKRI
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Solution-processed organometal trihalide perovskite solar cells are attracting increasing interest, leading to high performances over 15% in thin film architectures. Here, we probe the presence of sub gap states in both solid and mesosuperstructured perovskite films and determine that they strongly influence the photoconductivity response and splitting of the quasi-Fermi levels in films and solar cells. We find that while the planar perovskite films are superior to the mesosuperstructured films in terms of charge carrier mobility (in excess of 20 cm(2) V-1 s(-1)) and emissivity, the planar heterojunction solar cells are limited in photovoltage by the presence of sub gap states and low intrinsic doping densities.
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