Journal
ACS NANO
Volume 8, Issue 7, Pages 6739-6747Publisher
AMER CHEMICAL SOC
DOI: 10.1021/nn500504s
Keywords
graphene oxide; poly(dopamine); nanocomposite; interfacial adhesion; reinforcement; toughening; humidity sensing
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Funding
- Center for Advanced Soft Electronics under the Global Frontier Research Program through the National Research Foundation (NRF) - Ministry of Science, ICT and Future Planning (MSIE), Korea
- Ministry of Education (MOE)
- NRF through the BK21 Plus Program (META-material-based Energy Harvest and Storage Technologies) [10Z20130011057]
- Human Resource Training Project for Regional Innovation [2012H1B8A2026133]
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Poly(dopamine)-treated graphene oxide/poly(vinyl alcohol) (dG-0/PVA) composite films were made and characterized. G-0 was modified with poly(dopamine) in aqueous solution and then chemically reduced to yield poly(dopamine)-treated reduced G-0. A combination of hydrogen bonding, strong adhesion of poly(dopamine) at the interface of PVA and G-0 sheets, and reinforcement by G-0 resulted in increases in tensile modulus, ultimate tensile strength, and strain-to-failure by 39, 100, and 89%, respectively, at 0.5 wt % dG-0 loading of the PVA. The dG-0 serves as a moisture barrier for water-soluble PVA, and the dG-0/PVA composite films were shown to be effective humidity sensors over the relative humidity range 40-100%.
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