Journal
ACS NANO
Volume 8, Issue 8, Pages 8317-8322Publisher
AMER CHEMICAL SOC
DOI: 10.1021/nn502776h
Keywords
molybdenum disulfide; heterojunction solar cell; 2D material; monolayer; chemical vapor deposition
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We realized photovoltaic operation in large-scale MoS2 monolayers by the formation of a type-II heterojunction with p-Si. The MoS2 monolayer introduces a built-in electric field near the interface between MoS2 and p-Si to help photogenerated carrier separation. Such a heterojunction photovoltaic device achieves a power conversion efficiency of 5.23%, which is the highest efficiency among all monolayer transition metal dichalcogenide-based solar cells. The demonstrated results of monolayer MoS2/Si-based solar cells hold the promise for integration of 2D materials with commercially available Si based electronics in highly efficient devices.
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