Journal
ACS NANO
Volume 7, Issue 5, Pages 4449-4458Publisher
AMER CHEMICAL SOC
DOI: 10.1021/nn401053g
Keywords
field-effect transistor; MoS2; few-layer; electric double layer; Schottky barrier
Categories
Funding
- NSF [ECCS-1128297, EEC-0832785]
- Center for Nanophase Materials Sciences [CNMS2011-066]
- Directorate For Engineering
- Div Of Electrical, Commun & Cyber Sys [1128297] Funding Source: National Science Foundation
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We report the fabrication of ionic liquid (IL)-gated field-effect transistors (FETs) consisting of bilayer and few-layer MoS2. Our transport measurements indicate that the electron mobility mu approximate to 60 cm(2) V-1 s(-1) at 250 K in IL-gated devices exceeds significantly that of comparable back-gated devices. IL-FETs display a mobility increase from approximate to 100 cm(2) V-1 s(-1) at 180 K to approximate to 220 cm(2) V-1 s(-1) at 77 K in good agreement with the true channel mobility determined from four-terminal measurements, ambipolar behavior with a high ON/OFF ratio >10(7) (10(4)) for electrons (holes), and a near ideal subthreshold swing of approximate to 50 mV/dec at 250 K. We attribute the observed performance enhancement, specifically the increased carrier mobility that is limited by phonons, to the reduction of the Schottky barrier at the source and drain electrode by band bending caused by the ultrathin IL dielectric layer.
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