4.8 Article

Synthesis of Few-Layer GaSe Nanosheets for High Performance Photodetectors

Journal

ACS NANO
Volume 6, Issue 7, Pages 5988-5994

Publisher

AMER CHEMICAL SOC
DOI: 10.1021/nn300889c

Keywords

gallium selenide; nanosheets; photodetectors

Funding

  1. NSFC [61172001, 10874177]
  2. special funds for the Major State Basic Research of China [2009CB929301]
  3. Scientific Research Foundation for the Returned Overseas Chinese Scholars, State Education Ministry
  4. Fundamental Research Funds for Central Universities
  5. Chinese Program for New Century Excellent Talents in University
  6. Scientific User Facilities Division, Office of Basic Energy Sciences, U.S. Department of Energy

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Two-dimensional (2D) semiconductor nanomaterials hold great promises for future electronics and optics. In this paper, a 2D nanosheets of ultrathin GaSe has been prepared by using mechanical cleavage and solvent exfoliation method. Single- and few-layer GaSe nanosheets are exfoliated on an SiO2/Si substrate and characterized by atomic force microscopy and Raman spectroscopy. Ultrathin GaSe-based photodetector shows a fast response of 0.02 s, high responsivity of 2.8 AW(-1) and high external quantum efficiency of 1367% at 254 nm, indicating that the two-dimensional nanostructure of GaSe is a new promising material for high performance photodetectors.

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