Journal
ACS NANO
Volume 6, Issue 2, Pages 1438-1448Publisher
AMER CHEMICAL SOC
DOI: 10.1021/nn2042412
Keywords
fluorescence; bowtie nano-aperture; plasmonic; lifetime; scattering
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Funding
- National Natural Science Foundation of China [61008026, 10821062, 90921008]
- National Basic Research Program of China [2007CB307001, 2009CB-930504]
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We report experimental behaviors of polarization-dependent, plasmonlc-enhanced molecular fluorescence within isolated bowtie nano-apertures (BNAs) milled in aluminum films. BNAs provide efficient control of the fluorescent count rate per molecule and the decay lifetime of the molecules and provide an effective detection volume at the nanometer scale by tuning either the excitation light polarization or the BNA size. Interestingly, large BNAs (>300 nm) present high plasmonic-enhanced fluorescence efficiency and can simultaneously confine the detection volume below the subdiffraction limit. Numerical simulations were performed that agreed qualitatively with the experimental results. The BNAs have potential applications, especially for single-molecule biological analysis.
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