Journal
ACS NANO
Volume 5, Issue 10, Pages 8040-8048Publisher
AMER CHEMICAL SOC
DOI: 10.1021/nn202620u
Keywords
bioimaging; ratiometric; upconversion luminescence; Hg2+
Categories
Funding
- National Science Foundation of China [20825101, 91027004]
- MOST of China [2011AA03A407]
- Shanghai Sci. Tech. Comm. [11XD1400200, 1052 nm03400]
- Shanghai Leading Academic Discipline Project [B108]
- CAS/SAFEA International Partnership Program for Creative Research Teams
- [IRT0911]
Ask authors/readers for more resources
A chromophoric ruthenium complex-assembled nanophosphor (N719-UCNPs) was achieved as a highly selective water-soluble probe for upconversion luminescence sensing and bioimaging of intracellular mercury Ions. The prepared nanophosphors were characterized by X-ray powder diffraction (XRD), transmission electron microscopy (TEM), energy-dispersive X-ray analysis (EDXA), Fourier transform infrared spectroscopy (FTIR), and X-ray photoelectron spectroscopy (XPS). Further application of N719-UCNPs in sensing Hg2+ was confirmed by optical titration experiment and upconversion luminescence live cell Imaging. Using the ratiometric upconversion luminescence as a detection signal, the detection limit of Hg2+ for this nanoprobe in water was down to 1.95 ppb, lower than the maximum level (2 ppb) of He2+ in drinking water set by the United States EPA. Importantly, the nanoprobe N719-UCNPs has been shown to be capable of monitoring changes in the distribution of Hg2+ in living cells by upconversion luminescence bioimaging.
Authors
I am an author on this paper
Click your name to claim this paper and add it to your profile.
Reviews
Recommended
No Data Available