4.8 Article

Organic Photovoltaic Devices Using Highly Flexible Reduced Graphene Oxide Films as Transparent Electrodes

Journal

ACS NANO
Volume 4, Issue 9, Pages 5263-5268

Publisher

AMER CHEMICAL SOC
DOI: 10.1021/nn1015874

Keywords

reduced graphene oxide; organic photovoltaic devices; flexible electrodes; optical transmittance; bending-induced tensile stress

Funding

  1. MOE [RG 20/07]
  2. NRF [NRF-CRP2-2007-01]
  3. A*STAR [092 101 00641]
  4. Centre for Biomimetic Sensor Science at NTU in Singapore

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The chemically reduced graphene oxide (rGO) was transferred onto polyethylene terephthalate (PET) substrates and then used as transparent and conductive electrodes for flexible organic photovoltaic (OPV) devices. The performance of the OPV devices mainly depends on the charge transport efficiency through rGO electrodes when the optical transmittance of rGO is above 65%. However, if the transmittance of rGO is less than 65%, the performance of the OPV device is dominated by the light transmission efficiency, that is, the transparency of rGO films. After the tensile strain (similar to 2.9%) was applied on the fabricated OPV device, it can sustain a thousand cycles of bending. Our work demonstrates the highly flexible property of rGO films, which provide the potential applications in flexible optoelectronics.

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