Journal
ACS NANO
Volume 5, Issue 1, Pages 574-580Publisher
AMER CHEMICAL SOC
DOI: 10.1021/nn102704h
Keywords
light-emitting electrochemical cell; metal-free; flexible; solution processing; graphene; superyellow; PEDOT-PSS; doping; p-n junction
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Funding
- Kempestiftelserna
- Carl Tryggers Stiftelse
- Swedish Research Council (Vetenskapsradet)
- Knut and Alice Wallenberg Foundation
- National Science Foundation [ECS 0543867]
- Royal Society
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We report flexible and metal free light-emitting electrochemical cells (LECs) using exclusively solution processed organic materials and illustrate interesting design opportunities offered by such conformable devices with transparent electrodes. Flexible LEC devices based on chemically derived graphene (COG) as the., cathode and poly(3,4-ethylenedioxythiophene) mixed with poly(styrenesulfonate) as the anode exhibit a low turnon voltage for yellow light emission (V = 2.8 V) and a good efficiency 2.4 (4.0) cd/A at a brightness of 100 (50) cd/m(2). We also find that COG is electrochemically inert over a wide potential range (+1.2 to -2.8 V vs ferrocene/ferrocenium) and exploit this property to demonstrate planar LEC devices with COG as both the anode and the cathode.
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