Journal
ACS APPLIED MATERIALS & INTERFACES
Volume 4, Issue 11, Pages 5800-5806Publisher
AMER CHEMICAL SOC
DOI: 10.1021/am302077c
Keywords
porous carbon; celtuce leaves; supercapacitor; CO2 capture; biomass; KOH activation
Funding
- Chinese Academy of Sciences
- Youth Science Foundations of Gansu Province [1107RJYA274]
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Business costs and energy/environmental concerns have increased interested in biomass materials for production of activated carbons, especially as electrode materials for supercapacitors or as solid-state adsorbents in CO2 adsorption area. In this paper, waste celtuce leaves were used to prepare porous carbon by air-drying, pyrolysis at 600 degrees C in argon, followed by KOH activation. The as-prepared porous carbon have a very high specific surface area of 3404 m(2)/g and a large pore volume of 1.88 cm(3)/g. As an electroactive material, the porous carbon exhibits good capacitive performance in KOH aqueous electrolyte, with the specific capacitances of 421 and 273 F/g in three and two-electrode systems, respectively. As a solid-state adsorbent, the porous carbon has an excellent CO2 adsorption capacity at ambient pressures of up to 6.04 and 4.36 mmol/g at 0 and 25 degrees C, respectively. With simple production process, excellent recyclability and regeneration stability, the porous carbon that was derived from celtuce leaves is among the most promising materials for high-performance supercapacitors and CO2 capture.
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