Journal
CHEM
Volume 4, Issue 4, Pages 833-844Publisher
CELL PRESS
DOI: 10.1016/j.chempr.2018.01.007
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Funding
- National Science Foundation [CBET-1438007]
- Basic Energy Sciences program of the US Department of Energy (DOE) Office of Science [DE-SC0005397]
- Assistant Secretary for Energy Efficiency and Renewable Energy of the US DOE Office of Vehicle Technologies through the Advanced Battery Materials Research Program [DE-EE000762]
- Robert A. Welch Foundation [F-1066]
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The cycling performance at 60 degrees C of a Na2MnFe(CN)(6)/Na cell with a ceramic solid electrolyte is compared with that of a cell with an organic-liquid electrolyte operating at room temperature. Analysis of the electrode-electrolyte interfaces after charge-discharge cycling showed that a sodium-metal anode that wets the solid electrolyte can be plated and stripped reversibly dendrite free and that the dissolution of the cyano-perovskite Na2MnFe(CN)(6) cathode that occurs with an organic-liquid electrolyte is eliminated with the utilization of the solid electrolyte. This demonstration indicates that a high-energy-density and low-cost sodium rechargeable battery can be competitive for large-scale electric energy storage where both the anode and cathode problems are solved in an all-solid-state battery.
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