Journal
TOPICS IN CURRENT CHEMISTRY
Volume 376, Issue 1, Pages -Publisher
SPRINGER INTERNATIONAL PUBLISHING AG
DOI: 10.1007/s41061-018-0185-4
Keywords
Terahertz; Gas-phase molecular rotations; Liquid-phase molecular dynamics; Magnetic resonances
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Funding
- Office of Naval Research Grant [N00014-13-10509]
- Defense University Research Instrumentation Program Grant [N00014-15-1-2879]
- National Science Foundation Grants [CHE-1111557, CHE-1665383]
- Samsung Global Research Outreach program
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Multidimensional spectroscopy in the visible and infrared spectral ranges has become a powerful technique to retrieve dynamic correlations and couplings in wide-ranging systems by utilizing multiple correlated light-matter interactions. Its extension to the terahertz (THz) regime of the electromagnetic spectrum, where rich material degrees of freedom reside, however, has been progressing slowly. This chapter reviews some of the THz-frequency two-dimensional (2D) spectroscopy techniques and experimental results realized in recent years. Examples include gas molecule rotations, spin precessions in magnetic systems, and liquid molecular dynamics studied by 2D THz or hybrid 2D THz-Raman spectroscopy techniques. The methodology shows promising applications to different THz-frequency degrees of freedom in various chemical systems and processes.
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