Journal
ORGANIC CHEMISTRY FRONTIERS
Volume 5, Issue 11, Pages 1854-1858Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c8qo00314a
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Funding
- National Natural Science Foundation of China [21776148, 21505083]
- Natural Science Foundation of Shandong Province [ZR2016BM07]
- Key Research & Development Project of Shandong Province [2018GSF118224]
- Qingdao Special Research Foundation of Science and Technology [16-6-2-29-nsh]
- Talents of High Level Scientific Research Foundation of Qingdao Agricultural University [6631115015, 6631110309]
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Incredibly electrophilic keteniminium ions generated in situ were employed as powerful intermediates for cascade [1,5]-hydride transfer/cyclization, via which inert benzylic and non-benzylic C(sp(3))-H bonds without a directing group were directly functionalized to furnish complex polycycles in a single operation.
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