Journal
ORGANIC CHEMISTRY FRONTIERS
Volume 5, Issue 1, Pages 59-63Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c7qo00718c
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Funding
- National Natural Science Foundation of China [21502132]
- Natural Science Foundation of Jiangsu Province [BK20150316]
- Jiangsu Specially Appointed Professor Plan
- Priority Academic Program Development of Jiangsu Higher Education Institutions (PAPD)
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A scandium complex based on a new type of tridentate ligand enabled an atom- and step-economical C(sp(3))-H addition of N, N-dimethyl anilines to a variety of unactivated alkenes affording branched products for the first time. A cationic o-dimethylaminophenyl scandium species was isolated and confirmed as the catalytic intermediate in this transformation.
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