4.3 Article

Implementation of cross correlation for energy discrimination on the time-of-flight spectrometer CORELLI

Journal

JOURNAL OF APPLIED CRYSTALLOGRAPHY
Volume 51, Issue -, Pages 315-322

Publisher

INT UNION CRYSTALLOGRAPHY
DOI: 10.1107/S160057671800403X

Keywords

neutron diffraction; energy discrimination; cross-correlation technique; time-of-flight neutron beamlines

Funding

  1. Scientific User Facilities Division, Basic Energy Sciences, Office of Science, US Department of Energy
  2. Materials Sciences and Engineering Division, Basic Energy Sciences, Office of Science, US Department of Energy

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The CORELLI instrument at Oak Ridge National Laboratory is a statistical chopper spectrometer designed and optimized to probe complex disorder in crystalline materials through diffuse scattering experiments. On CORELLI, the high efficiency of white-beam Laue diffraction combined with elastic discrimination have enabled an unprecedented data collection rate to obtain both the total and the elastic-only scattering over a large volume of reciprocal space from a single measurement. To achieve this, CORELLI is equipped with a statistical chopper to modulate the incoming neutron beam quasi-randomly, and then the cross-correlation method is applied to reconstruct the elastic component from the scattering data. Details of the implementation of the cross-correlation method on CORELLI are given and its performance is discussed.

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