Journal
JOURNAL OF MATERIALS CHEMISTRY C
Volume 6, Issue 11, Pages 2618-2634Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c7tc05972h
Keywords
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Funding
- US NSF [1507170]
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Tunable, narrow-linewidth photoluminescence with nearly ideal quantum yields and solution processability make colloidal quantum dots (QDs) a unique class of emitters for a variety of applications including light-mitting diodes (LEDs). Wide color gamut and high color saturation that can be achieved with QDs along with recent advances in QD-LEDs motivate their use as large-area, patternable electroluminescent materials especially in displays. In this review, critical issues in performance and long-term stability of QD-LEDs, Cd-free compositions necessary for practical applications, lower-symmetry heterostructures that impart new capabilities, and unconventional fabrication approaches are discussed. As the current CdSe-based QD-LEDs approach their performance limits, emerging nanorod heterostructures, as exemplified by the double heterojunction nanorods (DHNRs), can extend efficiencies beyond these limits. Furthermore, enhancements in device lifetime and light detection/photovoltaic capabilities using the same high-performance DHNR-LEDs can allow exciting prospects for novel emissive displays. Such multifunctional LEDs that can be solution-processed into large-area, mulitcolor pixel arrays may fundamentally alter how we perceive, interact with and utilize display devices.
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