4.6 Article

A solvent-switched in situ confinement approach for immobilizing highly-active ultrafine palladium nanoparticles: boosting catalytic hydrogen evolution

Journal

JOURNAL OF MATERIALS CHEMISTRY A
Volume 6, Issue 14, Pages 5544-5549

Publisher

ROYAL SOC CHEMISTRY
DOI: 10.1039/c8ta01093e

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Funding

  1. International Joint Research Program for Innovative Energy Technology of the Ministry of Economy, Trade, and Industry (METI)

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A facile and effective solvent-switched in situ confinement approach (SSISCA) has been developed to immobilize ultrafine and clean Pd NPs of similar to 1.75 nm into a nanoporous carbon support. The Pd NPs in situ confined within the carbon nanopores possess high catalytic activity and selectivity for hydrogen evolution from formic acid with a recordhigh TOF of 9110 h(-1) at 60 degrees C.

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