Journal
JOURNAL OF MATERIALS CHEMISTRY A
Volume 6, Issue 25, Pages 11631-11663Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c8ta03358g
Keywords
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Funding
- National Natural Science Foundation of China [91534109, 21276257]
- Strategic Priority Research Program of the Chinese Academy of Sciences [XDA09010103]
- National Key Projects for Fundamental Research and Development of China [2016YFB0100104]
- Beijing Municipal Science and Technology Project [D171100005617001]
- Henan Province Science and Technology Cooperation Project [172106000061]
- Australian Research Council
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Developing the next-generation high-energy density and safe batteries is of prime importance to meet the emerging demands in electronics, automobile industries and various energy storage systems. High-voltage lithium-ion batteries (LIBs) and solid-state batteries (SSBs) are two main directions attracting increasing interest in recent years, due to their potential applications in the near future. In both kinds of batteries, the electrolytes play a pivotal role but also create several bottleneck problems. In this review, recent progress in designing electrolytes for high-voltage LIBs and SSBs is summarized. First, the solvents, additives, ionic liquids and superconcentrated salts strategies for constructing high-voltage liquid electrolytes are reviewed, and then the applications of inorganic solids, solid polymers, gels and ionic liquids in solid-state electrolytes are presented. Finally, the general design rules of the electrolytes and their current limitations and future prospects are briefly discussed.
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