Journal
RSC ADVANCES
Volume 8, Issue 24, Pages 13112-13120Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c8ra01384e
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Funding
- Creative Research Initiative Center for Self-powered Actuation in Korea
- National Research Foundation of Korea (NRF) - Ministry of Education [NRF-2017R1A6A3A04004987]
- DGIST R&D Program of Ministry of Science, ICT and Future Planning of Korea [17-NT-02]
- Air Force Office of Scientific Research [AOARD-FA2386-13-1-4119, FA9550-15-1-0089]
- Robert A. Welch Foundation [AT-0029]
- Australian Research Council [DP110101073]
- Ministry of Science & ICT (MSIT), Republic of Korea [17-NT-02] Funding Source: Korea Institute of Science & Technology Information (KISTI), National Science & Technology Information Service (NTIS)
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Asymmetric supercapacitors are receiving much research interests due to their wide operating potential window and high energy density. In this study, we report the fabrication of asymmetrically configured yarn based supercapacitor by using liquid-state biscrolling technology. High loading amounts of reduced graphene oxide anode guest (90.1 wt%) and MnO2 cathode guest (70 wt%) materials were successfully embedded into carbon nanotube yarn host electrodes. The resulting asymmetric yarn supercapacitor coated by gel based organic electrolyte (PVDF-HFP-TEABF(4)) exhibited wider potential window (up to 3.5 V) and resulting high energy density (43 W h cm(-2)). Moreover, the yarn electrodes were mechanically strong enough to be woven into commercial textiles. The textile supercapacitor exhibited stable electrochemical energy storage performances during dynamically applied deformations.
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