Journal
CATALYSIS SCIENCE & TECHNOLOGY
Volume 8, Issue 6, Pages 1517-1521Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c7cy02484c
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Funding
- Federal Ministry of Education and Research (BMBF)
- MANGAN research cluster [FKZ 03SF0508]
- Deutscher Akademischer Austauschdienst (DAAD)
- Consejo Nacional de Ciencia y Tecnologia (CONACyT)
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Electrochemical water splitting using non-noble metals as catalysts is of increasing importance for the future energy sector. In particular, efficient catalysts for the demanding oxygen evolution reaction present a major challenge. As a contribution to this field, tailored mesoporous hard template materials based on manganese phthalocyanine were prepared. The preparation method proved to be crucial to achieve suitable physicochemical properties as a basis for high catalytic activity. The materials show overpotentials between 490 and 590 mV at 10 mA cm(-2) This can be mainly attributed to efficient graphitization, high Mn dispersion and tailored oxidation states.
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